The substitution chemistry of a useful new synthon with neutral donor ligands. The reactions of [TcCl3(NNPh2)(PPh3)2] with phosphine ligands. The X-ray crystal structures of [TcCl2(NNPh2)(PMe2Ph)3][PF6], [TcCl(NNPh2)(dppe)2][PF6]2 and [TcCl2(NNPh2)(TRIPHOS)][BPh4]

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