Volume 21; Issue 3

Chemistry - A European Journal

Volume 21; Issue 3

1

Synthesis of a Pentasaccharide and Neoglycoconjugates Related to Fungal α-(1→3)-Glucan and Their Use in the Generation of Antibodies to Trace Aspergillus fumigatus Cell Wall

Komarova, Bozhena S., Orekhova, Maria V., Tsvetkov, Yury E., Beau, Remi, Aimanianda, Vishukumar, Latgé, Jean-Paul, Nifantiev, Nikolay E.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 769 KB

english, 2015

2

Synthesis of a Pentasaccharide and Neoglycoconjugates Related to Fungal α-(1→3)-Glucan and Their Use in the Generation of Antibodies to Trace Aspergillus fumigatus Cell Wall

Komarova, Bozhena S., Orekhova, Maria V., Tsvetkov, Yury E., Beau, Remi, Aimanianda, Vishukumar, Latgé, Jean-Paul, Nifantiev, Nikolay E.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 919 KB

english, 2015

3

Synthesis of New Porphyrin-Fullerene Dyads Capable of Forming Charge-Separated States on a Microsecond Lifetime Scale

Konev, Alexander S., Khlebnikov, Alexander F., Prolubnikov, Pavel I., Mereshchenko, Andrey S., Povolotskiy, Alexey V., Levin, Oleg V., Hirsch, Andreas

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 888 KB

english, 2015

4

Multivalency as a Key Factor for High Activity of Selective Supported Organocatalysts for the Baylis-Hillman Reaction

Goren, Kerem, Karabline-Kuks, Jeny, Shiloni, Yael, Barak-Kulbak, Einav, Miller, Scott J., Portnoy, Moshe

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 547 KB

english, 2015

5

Dual Photo- and pH-Responsive Supramolecular Nanocarriers Based on Water-Soluble Pillar[6]arene and Different Azobenzene Derivatives for Intracellular Anticancer Drug Delivery

Hu, Xiao-Yu, Jia, Keke, Cao, Yu, Li, Yan, Qin, Shan, Zhou, Fan, Lin, Chen, Zhang, Dongmei, Wang, Leyong

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 2.66 MB

english, 2015

6

Scalable Room-Temperature Synthesis of Mesoporous Nanocrystalline ZnMn 2 O 4 with Enhanced Lithium Storage Properties for Lithium-Ion Batteries

Yuan, Changzhou, Zhang, Longhai, Hou, Linrui, Zhou, Lu, Pang, Gang, Lian, Lin

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 810 KB

english, 2015

7

Functionalization of Quinoxalines by Using TMP Bases: Preparation of Tetracyclic Heterocycles with High Photoluminescene Quantum Yields

Nafe, Julia, Herbert, Simon, Auras, Florian, Karaghiosoff, Konstantin, Bein, Thomas, Knochel, Paul

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 757 KB

english, 2015

8

Reversible Multistimuli-Response Fluorescent Switch Based on Tetraphenylethene-Spiropyran Molecules

Qi, Qingkai, Qian, Jingyu, Ma, Suqian, Xu, Bin, Zhang, Sean Xiao-An, Tian, Wenjing

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.85 MB

english, 2015

9

Room-Temperature Synthesis of Cu 2− x E (E=S, Se) Nanotubes with Hierarchical Architecture as High-Performance Counter Electrodes of Quantum-Dot-Sensitized Solar Cells

Chen, Xin Qi, Li, Zhen, Bai, Yang, Sun, Qiao, Wang, Lian Zhou, Dou, Shi Xue

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 2.27 MB

english, 2015

10

Long-Lived Excited States of Zwitterionic Copper(I) Complexes for Photoinduced Cross-Dehydrogenative Coupling Reactions

Wang, Bin, Shelar, Deepak Prakash, Han, Xian-Zhu, Li, Ting-Ting, Guan, Xiangguo, Lu, Wei, Liu, Kun, Chen, Yong, Fu, Wen-Fu, Che, Chi-Ming

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 524 KB

english, 2015

11

Substituent and Solvent Effects on the Excited State Deactivation Channels in Anils and Boranils

Dobkowski, Jacek, Wnuk, Paweł, Buczyńska, Joanna, Pszona, Maria, Orzanowska, Grażyna, Frath, Denis, Ulrich, Gilles, Massue, Julien, Mosquera-Vázquez, Sandra, Vauthey, Eric, Radzewicz, Czesław, Ziessel

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 3.55 MB

english, 2015

12

Elucidating the Thermal Decomposition of Dimethyl Methylphosphonate by Vacuum Ultraviolet (VUV) Photoionization: Pathways to the PO Radical, a Key Species in Flame-Retardant Mechanisms

Liang, Shuyu, Hemberger, Patrick, Neisius, N. Matthias, Bodi, Andras, Grützmacher, Hansjörg, Levalois-Grützmacher, Joelle, Gaan, Sabyasachi

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 673 KB

english, 2015

13

Sulfur Encapsulated in a TiO 2 -Anchored Hollow Carbon Nanofiber Hybrid Nanostructure for Lithium-Sulfur Batteries

Zhang, Zhian, Li, Qiang, Jiang, Shaofeng, Zhang, Kai, Lai, Yanqing, Li, Jie

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.48 MB

english, 2015

14

Straightforward Synthesis of 1,2-Dicyanoalkanes from Nitroalkenes and Silyl Cyanide Mediated by Tetrabutylammonium Fluoride

Kiyokawa, Kensuke, Nagata, Takaya, Hayakawa, Junpei, Minakata, Satoshi

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 341 KB

english, 2015

15

Multicomponent Synthesis of Chiral Bidentate Unsymmetrical Unsaturated N -Heterocyclic Carbenes: Copper-Catalyzed Asymmetric CC Bond Formation

Jahier-Diallo, Claire, Morin, Marie S. T., Queval, Pierre, Rouen, Mathieu, Artur, Isabelle, Querard, Pierre, Toupet, Loic, Crévisy, Christophe, Baslé, Olivier, Mauduit, Marc

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 480 KB

english, 2015

16

Gold(I)/Chiral Brønsted Acid Catalyzed Enantioselective Hydroamination-Hydroarylation of Alkynes: The Effect of a Remote Hydroxyl Group on the Reactivity and Enantioselectivity

Shinde, Valmik S., Mane, Manoj V., Vanka, Kumar, Mallick, Arijit, Patil, Nitin T.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 624 KB

english, 2015

17

Versatile Bisethynyl[60]fulleropyrrolidine Scaffolds for Mimicking Artificial Light-Harvesting Photoreaction Centers

Kremer, Adrian, Bietlot, Emerance, Zanelli, Alberto, Malicka, Joanna M., Armaroli, Nicola, Bonifazi, Davide

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 834 KB

english, 2015

18

Selective and Sensitive Aqueous-Phase Detection of 2,4,6-Trinitrophenol (TNP) by an Amine-Functionalized Metal-Organic Framework

Joarder, Biplab, Desai, Aamod V., Samanta, Partha, Mukherjee, Soumya, Ghosh, Sujit K.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.62 MB

english, 2015

19

Differences and Comparisons of the Properties and Reactivities of Iron(III)-hydroperoxo Complexes with Saturated Coordination Sphere

Faponle, Abayomi S., Quesne, Matthew G., Sastri, Chivukula V., Banse, Frédéric, de Visser, Sam P.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 3.29 MB

english, 2015

20

Rhodium Bis(quinolinyl)benzene Complexes for Methane Activation and Functionalization

Fu, Ross, O'Reilly, Matthew E., Nielsen, Robert J., Goddard III , William A., Gunnoe, T. Brent

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.12 MB

english, 2015

21

Synthesis and Conformational Analysis of Hybrid α/β-Dipeptides Incorporating S -Glycosyl-β 2,2 -Amino Acids

García-González, Iván, Mata, Lara, Corzana, Francisco, Jiménez-Osés, Gonzalo, Avenoza, Alberto, Busto, Jesús H., Peregrina, Jesús M.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.36 MB

english, 2015

22

Palladium(0)-Catalyzed Single and Double Isonitrile Insertion: A Facile Synthesis of Benzofurans, Indoles, and Isatins

Senadi, Gopal Chandru, Hu, Wan-Ping, Boominathan, Siva Senthil Kumar, Wang, Jeh-Jeng

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 669 KB

english, 2015

23

Highly Sensitive INHIBIT and XOR Logic Gates Based on ICT and ACQ Emission Switching of a Porphyrin Derivative

Xu, Xiao-Ling, Lin, Fu-Wen, Xu, Wei, Wu, Jian, Xu, Zhi-Kang

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 839 KB

english, 2015

24

A Facile Top-Down Protocol for Postsynthesis Modification of Hierarchical Aluminum-Rich MFI Zeolites

Yu, Lili, Huang, Shengjun, Miao, Shu, Chen, Fucun, Zhang, Shuang, Liu, Zhenni, Xie, Sujuan, Xu, Longya

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.45 MB

english, 2015

25

113 Cd Solid-State NMR for Probing the Coordination Sphere in Metal-Organic Frameworks

Kuttatheyil, Anusree Viswanath, Handke, Marcel, Bergmann, Jens, Lässig, Daniel, Lincke, Jörg, Haase, Jürgen, Bertmer, Marko, Krautscheid, Harald

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 976 KB

english, 2015

26

Deciphering Ligands’ Interaction with Cu and Cu 2 O Nanocrystal Surfaces by NMR Solution Tools

Glaria, Arnaud, Cure, Jérémy, Piettre, Kilian, Coppel, Yannick, Turrin, Cédric-Olivier, Chaudret, Bruno, Fau, Pierre

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.37 MB

english, 2015

27

Synthesis, Structures, and Properties of Crystalline Salts with Radical Anions of Metal-Containing and Metal-Free Phthalocyanines

Konarev, Dmitri V., Kuzmin, Alexey V., Faraonov, Maxim A., Ishikawa, Manabu, Khasanov, Salavat S., Nakano, Yoshiaki, Otsuka, Akihiro, Yamochi, Hideki, Saito, Gunzi, Lyubovskaya, Rimma N.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 6.51 MB

english, 2015

28

Synthesis and Characterisation of Self-Assembled and Self-Adjuvanting Asymmetric Multi-Epitope Lipopeptides of Ovalbumin

Eskandari, Sharareh, Stephenson, Rachel J., Fuaad, Abdullah Ahmad, Apte, Simon H., Doolan, Denise L., Toth, Istvan

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.11 MB

english, 2015

29

Iron-Oxalato Framework with One-Dimensional Open Channels for Electrochemical Sodium-Ion Intercalation

Wang, Xianfen, Kurono, Ryosuke, Nishimura, Shin-ichi, Okubo, Masashi, Yamada, Atsuo

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.44 MB

english, 2015

30

Multiple-Stimulus-Responsive Supramolecular Gels of Two Components and Dual Chiroptical Switches

Miao, Wangen, Qin, Long, Yang, Dong, Jin, Xue, Liu, Minghua

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.30 MB

english, 2015

31

Chemoselective Bioconjugation of Triazole Phosphonites in Aqueous Media

Vallée, M. Robert J., Majkut, Paul, Krause, Dagmar, Gerrits, Michael, Hackenberger, Christian P. R.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 788 KB

english, 2015

32

Metal Complexes of a Boron-Dipyrromethene (BODIPY)-Tagged N-Heterocyclic Carbene (NHC) as Luminescent Carbon Monoxide Chemodosimeters

Kos, Pavlo, Plenio, Herbert

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 453 KB

english, 2015

33

A Regioselective Synthesis of Benzopinacolones through Aerobic Dehydrogenative α-Arylation of the Tertiary sp 3 CH Bond of 1,1-Diphenylketones with Aromatic and Heteroaromatic Compounds

More, Nagnath Yadav, Jeganmohan, Masilamani

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 507 KB

english, 2015

34

Silver/Gold Core-Shell Nanoprism-Based Plasmonic Nanoprobes for Highly Sensitive and Selective Detection of Hydrogen Sulfide

Yang, Xinjian, Ren, Yuqian, Gao, Zhiqiang

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.18 MB

english, 2015

35

(Metallo)porphyrins as Potent Phototoxic Anti-Cancer Agents after Irradiation with Red Light

Antoni, Philipp M., Naik, Anu, Albert, Ina, Rubbiani, Riccardo, Gupta, Susmita, Ruiz-Sanchez, Pilar, Munikorn, Pornkanok, Mateos, José M., Luginbuehl, Vera, Thamyongkit, Patchanita, Ziegler, Urs, Gass

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 669 KB

english, 2015

36

Unexpected Carbon Dioxide Inclusion in Water-Saturated Pores of Metal-Organic Frameworks with Potential for Highly Selective Capture of CO 2

Kim, Daeok, Lim, Hyung-Kyu, Ro, Hyeyoon, Kim, Hyungjun, Lee, Huen

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 728 KB

english, 2015

37

Molybdenum Complexes Supported by Mixed NHC/Phosphine Ligands: Activation of N 2 and Reaction With P(OMe) 3 to the First Meta -Phosphite Complex

Gradert, Christian, Stucke, Nadja, Krahmer, Jan, Näther, Christian, Tuczek, Felix

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 563 KB

english, 2015

38

Metal-Carbonyl Units for Vibrational and Luminescence Imaging: Towards Multimodality

Clède, Sylvain, Policar, Clotilde

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 2.44 MB

english, 2015

39

Asymmetric Synthesis of Fully Substituted Cyclopentane-Oxindoles through an Organocatalytic Triple Michael Domino Reaction

Zou, Liang-Hua, Philipps, Arne R., Raabe, Gerhard, Enders, Dieter

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 480 KB

english, 2015

40

Graphical Abstract: Chem. Eur. J. 3/2015

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 5.82 MB

english, 2015

41

Gold(I)-Catalyzed 1,2-Acyloxy Migration/[3+2] Cycloaddition of 1,6-Diynes with an Ynamide Propargyl Ester Moiety: Highly Efficient Synthesis of Functionalized Cyclopenta[ b ]indoles

Liu, Jun, Chen, Ming, Zhang, Liangwei, Liu, Yuanhong

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 304 KB

english, 2015

42

Molecular-Level Insights into Intrinsic Peroxidase-Like Activity of Nanocarbon Oxides

Zhao, Ruisheng, Zhao, Xiang, Gao, Xingfa

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 755 KB

english, 2015

43

Functional Carbazole Liquid-Crystal Block Codendrimers with Optical and Electronic Properties

Gracia, Ismael, Feringán, Beatriz, Serrano, José Luis, Termine, Roberto, Golemme, Attilio, Omenat, Ana, Barberá, Joaquín

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.53 MB

english, 2015

44

Solution Polymeric Optical Temperature Sensors with Long-Term Memory Function Powered by Supramolecular Chemistry

de la Rosa, Victor R., Hoogenboom, Richard

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.98 MB

english, 2015

45

Frontispiece: Synthesis, Structures, and Properties of Crystalline Salts with Radical Anions of Metal-Containing and Metal-Free Phthalocyanines

Konarev, Dmitri V., Kuzmin, Alexey V., Faraonov, Maxim A., Ishikawa, Manabu, Khasanov, Salavat S., Nakano, Yoshiaki, Otsuka, Akihiro, Yamochi, Hideki, Saito, Gunzi, Lyubovskaya, Rimma N.

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 5.29 MB

2015

46

Back Cover: Room-Temperature Synthesis of Cu 2− x E (E=S, Se) Nanotubes with Hierarchical Architecture as High-Performance Counter Electrodes of Quantum-Dot-Sensitized Solar Cells (Chem. Eur. J. 3/2015)

Chen, Xin Qi, Li, Zhen, Bai, Yang, Sun, Qiao, Wang, Lian Zhou, Dou, Shi Xue

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 759 KB

2015

47

High Ionic Conductivity in a LiFeO 2 -LiAlO 2 Composite Under H 2 /Air Fuel Cell Conditions

Lan, Rong, Tao, Shanwen

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.15 MB

english, 2015

48

Bioinspired Copper(I) Complexes that Exhibit Monooxygenase and Catechol Dioxygenase Activity

Arnold, Aline, Metzinger, Ramona, Limberg, Christian

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 853 KB

english, 2015

49

Insights into the Crystallisation Process from Anhydrous, Hydrated and Solvated Crystal Forms of Diatrizoic Acid

Fucke, Katharina, McIntyre, Garry J., Lemée-Cailleau, Marie-Hélène, Wilkinson, Clive, Edwards, Alison J., Howard, Judith A. K., Steed, Jonathan W.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.60 MB

english, 2015

50

Can CH⋅⋅⋅π Interactions Be Used To Design Single-Chain Magnets?

Singh, Mukesh Kumar, Rajaraman, Gopalan

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 758 KB

english, 2015

51

Specificity of Furanoside-Protein Recognition through Antibody Engineering and Molecular Modeling

Lak, Parnian, Makeneni, Spandana, Woods, Robert J., Lowary, Todd L.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.39 MB

english, 2015

52

Cover Picture: Synthesis of a Pentasaccharide and Neoglycoconjugates Related to Fungal α-(1→3)-Glucan and Their Use in the Generation of Antibodies to Trace Aspergillus fumigatus Cell Wall (Chem. Eur. J. 3/2015)

Komarova, Bozhena S., Orekhova, Maria V., Tsvetkov, Yury E., Beau, Remi, Aimanianda, Vishukumar, Latgé, Jean-Paul, Nifantiev, Nikolay E.

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 356 KB

2015

53

Inside Back Cover: A Facile Top-Down Protocol for Postsynthesis Modification of Hierarchical Aluminum-Rich MFI Zeolites (Chem. Eur. J. 3/2015)

Yu, Lili, Huang, Shengjun, Miao, Shu, Chen, Fucun, Zhang, Shuang, Liu, Zhenni, Xie, Sujuan, Xu, Longya

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 768 KB

2015

54

Inside Cover: Insights into the Crystallisation Process from Anhydrous, Hydrated and Solvated Crystal Forms of Diatrizoic Acid (Chem. Eur. J. 3/2015)

Fucke, Katharina, McIntyre, Garry J., Lemée-Cailleau, Marie-Hélène, Wilkinson, Clive, Edwards, Alison J., Howard, Judith A. K., Steed, Jonathan W.

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 611 KB

2015

55

Metalation Kinetics of the Human α-Metallothionein 1a Fragment Is Dependent on the Fluxional Structure of the apo-Protein

Irvine, Gordon W., Duncan, Kelly E. R., Gullons, Meredith, Stillman, Martin J.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.27 MB

english, 2015

56

Fluorination of Isotopically Labeled Turbostratic and Bernal Stacked Bilayer Graphene

Ek Weis, Johan, Costa, Sara D., Frank, Otakar, Bastl, Zdenek, Kalbac, Martin

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.19 MB

english, 2015

57

Oxoanionic Noble Metal Compounds from Fuming Nitric Acid: The Palladium Examples Pd(NO 3 ) 2 and Pd(CH 3 SO 3 ) 2

Bruns, Jörn, Klüner, Thorsten, Wickleder, Mathias S.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 859 KB

english, 2015

58

Frontispiece: Molecular-Level Insights into Intrinsic Peroxidase-Like Activity of Nanocarbon Oxides

Zhao, Ruisheng, Zhao, Xiang, Gao, Xingfa

Journal:

Chemistry - A European Journal

Year:

2015

File:

PDF, 609 KB

2015

59

Silver-Free Activation of Ligated Gold(I) Chlorides: The Use of [Me 3 NB 12 Cl 11 ] − as a Weakly Coordinating Anion in Homogeneous Gold Catalysis

Wegener, Michael, Huber, Florian, Bolli, Christoph, Jenne, Carsten, Kirsch, Stefan F.

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 508 KB

english, 2015

60

Spotlights on our sister journals: Chem. Eur. J. 3/2015

Journal:

Chemistry - A European Journal

Year:

2015

Language:

english

File:

PDF, 1.90 MB

english, 2015